Supplementary material pdf file

The supplementary material includes logistic fits for trajectories T1-T5, parameters a, τc, and r obtained by curve-fitting simulated data to the logistic function, characterization of the patches in the 170 K MD simulation, residence time of the molecules in the HDL-like phase for trajectories T1-T3 and T5. Patches characterization and residence time for the 170 K MD simulation of the 710 water molecules box. Figures analogous to Figure 6 for trajectories T1-T3 and T5. Density of the initial structure; logistic fits for trajectories T1B and T2B, parameters a, τc, and r obtained by curve-fitting simulated data to the logistic function, fraction of HDL-like molecules at time 0, average NTC value at time 0, τ1 and τ2 for trajectories T1B and T2B; residence time of the molecules in the HDL-like phase for trajectories T1B and T2B; figures analogous to Figure 6 for trajectories T1B and T2B. Time evolution of the HDL fraction and patches investigation for the trajectory in proximity to the critical point.