posted on 2024-10-18, 12:05authored byGuillaume Le Breton, Claire Loison, Kevin Vynck, Emmanuel Benichou, Oriane Bonhomme
A. Reminders of the response theory
B. Separation of the polarization density into different terms
C. Quadrupolar hyperpolarizability in the liquid phase
D. Number of QM/MM calculations per altitude
E. ai coefficients to fit polarization-resolved S-SHG experiments
F. Variation of the dipole second hyperpolarizability components in the laboratory frame
G. Change in polarization-resolved SHG intensity with the optical index of the interface