Supplementary Material: Freezing line of polydisperse hard spheres via direct coexistence simulations

Additional details for the generation of the deterministic particle size distribution as well as derivations for the effect of particle size on the free energy can be found in the supplementary material available online. We also provide the derivation for the equations of motions in the semi-grand canonical ensemble, as well as implementation details for the EDMC approach. An overview of the effects of system size on the determination of coexistence conditions is also provided, along with additional details on the phase composition of the system at coexistence, and the excess surface absorption for the FCCb interface.