S1, S2, S3, S4, S5, S6, S7, S8

Supplementary Information S1 - Convergence of heat capacity by multiple histogram technique of Al55 at different timesteps. Supplementary Information S2 - Convergence of heat capacity by multiple histogram technique of Al53 at different timesteps. Supplementary Information S3 - Lindemann index for Al53: (a) individual atoms and (b) averaged. Supplementary Information S4 - Lindemann index for Al60: (a) individual atoms and (b) averaged. Supplementary Information S5 - Lindemann index for Al116: (a) individual atoms and (b) averaged. Supplementary Information S6 - Lindemann index for Al128: (a) individual atoms and (b) averaged. Supplementary Information S7 - Comparison of Latent Heat: Experimental vs. Com- puted Data. Supplementary Information S8 - Comparison of entropy change: Experimental vs. Computed Data.