Supplementary materials

See the supplementary materials for additional information on the sample preparation, experimental section, calculation method, analysis of ARPRS, AFM, OM, ARPRS of MoS2 nanosheets and CrOCl nanoflake, Plane-averaged differential charge density of MoS2/CrOCl heterostructure, calculated band structure of CrOCl, OM, AFM, SEM and Raman of MoS2/CrOCl heterostructure prepared by dry transferred method, full spectra of ARPRS and ARPPLS of twisted MoS2/CrOCl heterostructure, ARPRS of twisted MoS2/CrOCl heterostructure with various thickness of CrOCl, AFM of 55{degree sign} twisted heterostructure.